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This book covers polymer electrolyte membranes PEMs from fundamentals to applications, describing their structure, properties, synthesis, and use in electrochemical energy storage and solar energy conversion technologies. The text discusses cutting-edge methodologies in PEM material selection and fabrication, providing an overview of the state of the art of PEM development, while pointing out important challenges and recommending mitigation strategies to improve PEM performance. It analyzes the current integration of PEMs with primary power devices and considers future research trends for the next generation of PEMs.